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Review Article

Recent Advancements in High-Performance Solid Electrolytes for Li-ion Batteries: Towards a Solid Future

Author(s): Imran Murtaza, Muhammad Umair Ali, Hongtao Yu, Huai Yang, Muhammad Tariq Saeed Chani*, Khasan S. Karimov*, Hong Meng*, Wei Huang and Abdullah M. Asiri

Volume 16, Issue 4, 2020

Page: [507 - 533] Pages: 27

DOI: 10.2174/1573413716666191230153257

Price: $65

Abstract

With the emergence of non-conventional energy resources and development of energy storage devices, serious efforts on lithium (Li) based rechargeable solid electrolyte batteries (Li- SEBs) are attaining momentum due to their potential as a safe candidate to replace state-of-the-art conventionally existing flammable organic liquid electrolyte-based Li-ion batteries (LIBs). However, Li-ion conduction in solid electrolytes (SEs) has been one of the major bottlenecks in large scale commercialization of next-generation Li-SEBs. Here, in this review, various challenges in the realization of high-performance Li-SEBs are discussed and recent strategies employed for the development of efficient SEs are reviewed. In addition, special focus is laid on the ionic conductivity enhancement techniques for inorganic (including ceramics, glasses, and glass-ceramics) and polymersbased SEs. The development of novel fabrication routes with controlled parameters and highperformance temperature optimized SEs with stable electrolyte-electrode interfaces are proposed to realize highly efficient Li-SEBs.

Keywords: Solid electrolytes, Li-ion, solid-state batteries, ionic conductivity, electrolyte-electrode interface, electrochemical performance, energy storage devices.

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