Title:Recent Advancements in High-Performance Solid Electrolytes for Li-ion Batteries: Towards a Solid Future
VOLUME: 16 ISSUE: 4
Author(s):Imran Murtaza, Muhammad Umair Ali, Hongtao Yu, Huai Yang, Muhammad Tariq Saeed Chani*, Khasan S. Karimov*, Hong Meng*, Wei Huang and Abdullah M. Asiri
Affiliation:Institute of Advanced Materials, Nanjing Tech University, Nanjing 211816, Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing 100871, Institute of Advanced Materials, Nanjing Tech University, Nanjing 211816, Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing 100871, Center of Excellence for Advanced Materials Research, King Abdulaziz University, Jeddah 21589, P.O. Box 80203, Ghulam Ishaq Khan Institute of Engineering Sciences and Technology, Topi-23640, District Swabi, KPK, Institute of Advanced Materials, Nanjing Tech University, Nanjing 211816, Institute of Advanced Materials, Nanjing Tech University, Nanjing 211816, Center of Excellence for Advanced Materials Research, King Abdulaziz University, Jeddah 21589, P.O. Box 80203
Keywords:Solid electrolytes, Li-ion, solid-state batteries, ionic conductivity, electrolyte-electrode interface, electrochemical
performance, energy storage devices.
Abstract:With the emergence of non-conventional energy resources and development of energy
storage devices, serious efforts on lithium (Li) based rechargeable solid electrolyte batteries (Li-
SEBs) are attaining momentum due to their potential as a safe candidate to replace state-of-the-art
conventionally existing flammable organic liquid electrolyte-based Li-ion batteries (LIBs). However,
Li-ion conduction in solid electrolytes (SEs) has been one of the major bottlenecks in large scale
commercialization of next-generation Li-SEBs. Here, in this review, various challenges in the realization
of high-performance Li-SEBs are discussed and recent strategies employed for the development
of efficient SEs are reviewed. In addition, special focus is laid on the ionic conductivity enhancement
techniques for inorganic (including ceramics, glasses, and glass-ceramics) and polymersbased
SEs. The development of novel fabrication routes with controlled parameters and highperformance
temperature optimized SEs with stable electrolyte-electrode interfaces are proposed to
realize highly efficient Li-SEBs.